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Kind of a big topic, since I don't know exactly what genres you're looking for, but here's some that I highly recommend:
Rozen Maiden: Supernatural, dramatic, action, comedy
Elfen Lied: Supernatural, dramatic, action, psychological, horror, romance
Kamisama Kazoku: Supernatural, dramatic, romance, comedy
Angel Beats!: Supernatural, action
Hope you haven't already seen all of those! They're all some of my favorite series.
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