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Hmm, maybe Sayonara Zetsubou Sensei? It likes to play with patterns, sudden color changes, art shifts, also the content is very unique.
Have only seen La Maison en Petits Cubes (loved that one, really distinctive style and the enactment was great), Voices of a distant star(did you know the whole thing was made by one person?), 5 centimeters per second (most detailed Animation I've ever seen) and Serial Experiments Lain (very confusing but interesting art and theme).
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