Seconding ToL, ToA, the Shadow Hearts games, Suikoden V, and DDS.
The Shadow Hearts games have become more animu styled over the years, but since you said you liked that I'd say it's a good reccomedation. I wish for another game like Koudelka...
Also, I reccomend the original Persona trilogy. The original Persona games had a good mix between story and characters, my favorite being Eternal Punishment because it's cast is full of mature adults, for once. (Persona 3 then did a 180.)
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