I think "4 girls and a idol" will be one of the best chapter to adapt for the OVA, because undoubtedly, it signal the return of earlier girls, and on how this show will not entirely follow the "monster girl of the week" method...
Other than the obvious Tenri arc, S3 if would be confirmed gonna be really interesting if they play on the melancholy Keima had after Manami arc. And also melodrama of Reiko chapter. Maybe also put a heavy tone on Sumire's family issue? They were success with Chihiro arc afterall
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