If I didn't give away a Manga or Anime DVD it would be an all time favorite to me.
Manga:
Hayate no Gotoku (start with the top and the series is not yet complete)
Negima (same thing not finished yet)
Strawberry 100% (working on finishing this series)
Samauri Girl Real Bout High School (First series I bought and completed and I still am holding on to)
To-Love-Ru caught my interest (untranslated) so it's an honorable mention
Anime:
No matter what I said that I wouldn't touch horror series, due to the story line, where they based the series from and some comedy this is my series hands down:
Chrono Crusade
Hayate no Gotoku has become a close second rather than a distant second
Full Metal Panic (1st Season) is a distant third
I have other keepers but they're not even close to third
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