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Just wondering but was the earliest tsundere Ayaka Morikawa (I think) from Kimagure Orange Road?
That's the oldest series that I can think of that had such an active Tsundere character.
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My Favorite Anime Quotes Courtesy of Answerman of ANN:
1) By and Large...they are ** and *****.
2) What kind of girls do Anime Otaku males want? ..................... Female.
3) The odds are good, that the goods are odd.
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