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Without much humour you say...
Usagi Drop is an ongoing show and does have jokes and stuff but I would call it quiet mature since jokes are not stupid like in usual animes.
Aoi Bungaku series are set of small stories, each is different. The longest is 4 episodes long. Each story covers some seriouse topic.
Bungaku Shoujo was quiet mature.
Clannad does have animes standard humour but over all it covers some mature topics.
Claymore doesn't have much humour.
Elfen Lied is mature with a lot of blood and nudity but not hentai.
Ga-Rei Zero has some random humour in some episodes but eventually takes darker and mature colours.
Ghost Hunt has a bit of humour to take down tension but it never ruins seriouse moments.
GTO is full of humour but despite that it covers quiet seriouse and mature topics.
Hakuouki doesn't have the standard anime jokes and is quiet mature.
Kanon 2006 does have humour but just like Clannad covers some seriouse topics,
Monster is mature.
Phantom: Requiem for the Phantom and Rainbow: Nisha Rokubou no Shichininperfectly meet the bill.
Shiki are mature series.
Sword of the stranger
Wolf's Rain
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