Well that doesn't tell much about your specific taste, so it's hard to pick; i've seen so many good ones.
Well, from a time-line basis...
YuYuHakusho.
Saint Seiya (Though I've been pissed off with it for a couple years, I was a fanboy until 10-12 years of age.)
Since the list would go for a long time, and I definetly don't have that much skin on my fingertips, here's some of the newest ones:
Full Metal Alchemist
Full Metal Panic / Fumoffu / The Second Raid
Rozen Maiden / Traumend
Genshiken (It's not finished, but it's a nice, funny and tr00 series.)
Elfen Lied (Don't watch if your stomach isn't up to the challenge.)
It's so hard to remember series you've watched when you need it, lol.
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Sometimes I look back and think to myself, "how the hell did I manage to screw this up?"
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