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Code Geass - For Lelouch alone, this is a must see anime, but the entire series was awesome. Episodes 23-25 were powerful.
The Melancholy of Haruhi Suzumiya - Kyon and Haruhi are by far the best male/female leads there. The show makes you laugh and think. Kyon's narration is awesome beyond words.
Tengen Toppa Gurren Lagann - Epic, Epic, Epic, Epic, Epic. Enough said.
Bleach (Till the end of the SS arc) - Doesn't break the mold, but it was just exciting to watch. Not many things got my blood pumping like Bleach.
Kanon 2006 - Beautiful story.
Rurouni Kenshin - Kenshin was awesome, great fights, classic.
Rurouni Kenshin: Tsuiokuhen - It was a work of art and awesome for completely different reasons to the TV series.
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