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I second the suggestions for Great Teacher Onizuka and Futakoi Alternative.
Other 'gems' I suggest are:
Azumanga Daioh - If you haven't seen this yet, slap yourself and watch it after GTO and Futakoi Alt.
Kiddy Grade - Now this is a real gem, ignore the "fanservice" that people called the first few episodes and stick to the end, you'll love it. It's about a girl who never dies dealing her tainted past.
Scrapped Princess - On her 16th birthday, this girl will bring destruction to the world. Drama follows as she and her siblings deal with the country hunting them, people that want the world to end, and friends that look at them differently when they find out who she is.
Midori no Hibi - A nice short 13 episode series. It's about a delinquent/yankee that is most feared in his school yet he can't get a girl for his life. Next morning, he wakes up and finds a girl on his right hand. Comedy and drama follows the duo.
Tsukuyomi ~Moon Phase ~ - An occult photographer goes and visits an old German castle, there he sees a girl sitting on rooftop by the visible full moon. Awestruck, he proclaimed he has to take a picture of her and when he tries to, she disappears. When he comes back with a few colleagues to take pictures of the girl. There he discovers a few things: the girl is a vampire, she 'kissed' him, she wants him to call her "master", and shes going to live with him to find her mother.
Iriya no Sora, UFO no Natsu - A short 6 episode OVA about a guy meets girl. However, that girl lives in a world that he can't even begin to imagine and she tells him, a war is about to start. Thus begins the heart-rending "UFO summer".
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