For your OP, I recommend
Spice and Wolf
&
She the Ultimate weapon.
These two anime really made me cry and feel other sorts of emotion. As did elfen lied however it's been said more than once, plus you listed it as mainstream and something you don't want.
As for your previous post, I enjoyed Claymore and Seto no hanayome is just amazing. Such an underated series. I hope you enjoy these.
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