Top of the list is the classic Grave of the Fireflies for me.
Saikano was pretty sad and Makoto Shinkai's films (Voices of a Distant Star, 5 Centimeters per Second).
Alien Nine was sad until I read the manga which carried on where the anime left off.
Quote:
Originally Posted by Wordplay
It might be this one: LINK.
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Oook that was strange.