I will second the Princess Tutu recommendation... Great show.
Cosmic Baton Girl Comet-san is very cute, and while aimed at a young audience, it can be quite entertaining, though it is fairly typical magical girl stuff.
Full Moon wo Sagashite is heart-warming/heart-wrenching. The story is really good (though fair warning, the songs get repeated way too much.)
Kita-he is brand new, and is geared towards an older audience. It is about relationships, and a new woman is focused on every couple of episodes.
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