if u haven't seen NHK yet, i would second on that, i started reading the manga a while back and it was actually the reason i found these forums a while back. real mature stuff, a real good suggestion
Samurai Champloo is a good anime, but man, it gets slow at times. still comical tho.
Paranoia agent is also great, but be ready to think, and i mean think deep, like English professor deep, there are so many subtle remarks and stuff, that if your not careful, at the end your not really sure who the real enemy is...
If u liked Bebop, Trigun is an old classic that a lot of people forget
Also, one of my personal favorite Excel Saga, is a completely random ass anime that has some maturity in it, as well as comedy and action. and some tongue in cheek romance. done by one of my Heros, Nabashin (who i actually got to meet and shake hands with at A-Kon in Dallas, sooooooooooooooo exciting!!!!!!!)
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