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I believe Casshern Sins and Soul Eater have some of the best tracks ever. Black Star's Theme song is most likely the best theme I've ever heard in an anime following Hiei's (Yu Yu Hakusho). The first season for Higurashi No Naku Koro Ni also has one of the best openings and endings. Yu Yu Hakusho itself also has some of the most fitting theme songs and excellent opening and ending.
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