I'll move this into the Suggestions forum, as it seem more appropriate than here. I'm not to sure if you are asking for DVDs releases only or if you would like the suggestions to include fansubs. But one advantage with fansubs is that at least you can download a couple of episodes and sample the series to see if it's what you're looking for.
As for suggestions from the available series you can download...
Shingetsutan Tsukihime
Condor Hero
Of the more recent licensed series (which you will not find as fansubs), maybe
Last Exile
Read or Die (OVA and TV)
Kaze no Yojimbo
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