Chrono Crusade's ending might make you cry, but I'm not sure if you want to get through 2 cours of action to see it. But you might, since you liked Elfen Lied (I think). Cross Game is good too, yeah.
SaiKano came closest to breaking me. Certain moments in Air made me teary. Grave of the Fireflies isn't for everyone, but I'll second it. Clannad wrecked me around episodes 7 and 9.
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