I second all those above...
Also try
Ai Yori Aoshi - its a bit like a harem, but the relationship between the 2 main characters is really really sweet
Aishiteruze Baby - sweet anime about a playboy who is forced to look after his little cousin
DN Angel - has both action and romance elements
Fruits Basket
Full Moon wo Sagashite - touching story about a girl who aspires to be a singer due to a promise with her childhood friend
Fushigi Yuugi - quite dated but good
Hoshi no Koe - very short and touching OVA from the director of 5cm per second
School Rumble
La Corda d'oro - an anime also revolving around music
Suzuka - sports and romance
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