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I think someone mentioned Fate/Stay Night, I supposed since you watched shakugan no shana you would like it too but it's a bit more drama and action focused.
For good storylines, Air or any other key work would be pretty good they're half drama/half romance bit more of the drama side. Also try KGNE if you like that genre
Da capo and it second season if you just want something light hearted to watch (its a harem anime).
and if you watch fate/stay night and like it you might also consider tsukihime, less comedy and kinda darker mood compared to f/sn though.
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