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As far as I understand Valeri does not lead any faction, quite the contrary, she is more like a prisoner of her own family. I do not think any pure blood vampire will joining the Harem, they are too proud and arrogant to fall for a reincarnated devil, they definitely do not match Isse.
I believe that something will happen with Rias’s delegation when she is visiting the territory of vampires, so the Gremori group will go in search of their missing comrades, somehow battling vampires and bring Valeri as "spoils of war ".
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