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VN:
Muv Luv. As improbable and risky as it is, but one can dream...
Saya no Uta, because I want dem beasts animated.
Manga:
Akame ga Kiru for me as well. It's just awesome with those character designs and I think the story structure would fit an anime well.
GATE. Because it would be awesome.
Most of all, though, Blame. Megastructures would be given justice if animated. Though it would be a very quiet series.
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