Wow, top 5 of all time. Trying to think of the top 5 is hard. I'll pick my favorites that I recommend to my friends who watch anime.
Akira - You just have to see it...
Trigun - My favorite anime overall because it's so watchable
Escaflowne - I liked the series, but not the movie (I saw the series first)
Cowboy Bebop - Well, it seems that everyone who watches anime series seems to watch Cowboy Bebop
Hellsing - I'm a fan of the vampire animes...
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