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Since you liked the NGE series I'd throw in Rahxephon
Other completed shows I'd recommend:
Darker than Black (not certain where the DVD releases are atm but I think it finished airing in USA its def licensed and a good show)
Cowboy Beebop, older show but also very nice. Like darker than black has good character development and story
Wolf's Rain
and maybe Eureka 7
I must add that Trinity Blood is a fair show to watch, the manga is a lot better but it is still enjoyable.
Also I'm not certain if this would count for you as licensed but Xam'd lost memories is a show licensed and released through the playstation3 store, it is also something you might want to check out. Sorry but it isn't on any dvd release yet in America nor does it air on TV in dub
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