Mushishi: makes you feel sad and melancholic, but like Kanon, there's a hopeful feel to it.
Zegapain: don't be fooled by its mecha-action scenes, the story develops slowly and when you realise what the real deal is about, you'll come to feel Zegapain (translated as: great pain). I don't think I cried while watching this anime, but there was certainly this heavy feeling of hopelessness throughout the series. Felt like the weight of the entire world was on your shoulders.
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