After listening to a few samples, I definitely think "dreamenddischarger" is my favorite episode four track. I think it uses the violin and electric guitar (?) well.
"Happy Maria" also deserves recognition for its eerie vocals. I cannot fully comprehend the lyrics, though.
Outside of episode four, I really like "Hane" and "Tekuteku". "Hane" for its lively piano composition and "Tekuteku" for its melancholic violin composition.
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