anime for your younger siblings eh?
I have a younger Sister myself that likes anime, here are some the ones she likes(be it Subed or Dubed on TV):
Aishiteruze Baby
Hunter x Hunter
Remi the nobody's girl(I think that was the title....don't remember...)
Romio's Blue Sky
Prince of Teniss
One Piece
Digimon
Detective Conan
Aka-Chan to Boku
can't think of anything else she likes...aslo, she liked Naruto and Pita Ten but you already have those =P
Also, you might want to try Konjiki no Gash Bell and Groove Adventure Rave , me thinks they'll like it =)
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