You might be stunned not to have seen these:
Future Boy Conan (can't recommend this highly enough)
Rurouni Kenshin: Tsuiokuhen
GitS: SAC
Kino no Tabi
Serial Experiments Lain
Monster
Master Keaton
Princess Tutu
Trigun
Taste tends to vary even more for comedies, but it appears you haven't seen any of my 5 favorites:
School Rumble
Azumanga Daioh
Irresponsible Captain Tylor
Kazemakase Tsukikage Ran
Full Metal Panic!
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