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most of the better series were listed by other users including Simoun, Juuni Kokki, Haibane Renmei, Kara no Kyoukai and Monster (all in my top 20 btw).
Some other series you might want to check out are Towards the Terra (The TV series) and Tatakau Shisho: The Book of Bantorra , both are Sci-fi/Mystery series with some good character development and interesting settings.
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