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My favourite Soundtracks as a whole, as in including vocal and background songs, are:
- .hack// series
- ef - A Tale of Two (Memories/Melodies)
- Video Girl AI
And basically any Yuki Kajiura soundtrack.
Now I have some other favourites, but those are mostly about vocal songs, not just OP/EDs, but Insert, Image and Character songs.
Then again, they aren't really based on a certain series, but mostly on the artists, since I might not like some of the other songs from that series, for example Bleach, with so many OP/EDs, not all are of my taste.
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