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Most of shounen to be honest... such as FMA, Soul Eater, D.Gray Man, Inuyasha, Hunter x Hunter, Katekyo Hitman Reborn!, Magi and etc.
More childish: Pokemon and Sonic. Dennou Coil is meant for younger audience. Phi Brain: Kami no Puzzle was quiet childish.
If you don't mind sport series, you can try Major.
Rozen Maiden, dolls come to live and fight each other.
Seirei no Moribito - amazing series but depends on how old your brother is since he simply might not appreciate it as much as you. Otherwise really worth it. Good action and no fan service.
Great story and characters.
Sengoku Basara
Senjou no Valkyria: Gallian Chronicles
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