If Sayaka was anything before her breakdown, it was that she was very passionate about being a hero and her love. Sure that's what ultimately led her to become broken, but I think one would have to be hard pressed to find anything to point to her being unstable before her meeting with Kyoko (who ended up rubbing Sayaka the wrong way through out the fight, and when she ended up being saved by Homura to boot ... well, she was certainly quite upset by how powerless she was in front of two she thought were rotten)
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