My favourite soundracks from anime are the ones for;
"X"
Death Note
Gun X Sword
Azumanga Daioh
Suzumiya Haruhi no Yuutsu
Fullmetal Alchemist
I liked the Azumanga Daioh one because it was so unique and clever, the way they used sounds such as hitting kettles, to make it suit the atmosphere of the anime.
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