For major plot-twisters I suggest Fullmetal Alchemist: Brotherhood, and after watching it (once it's finished), watch the original run from episode 17 onwards again.
I smell the absence of a Death Note, so check that one out too, it's GEASS-like but without the mecha and corny-ness.
Vampire knight has many twists as well, but I wouldn't rate the manga very highly and I haven't watched the anime...you can give it a shot though.
Casshern SINS- was a good show, no real twists around but still felt good watching it.
P.S: also watching monster atm, here comes ep.22!
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