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Baccano! if you don't mind a bit more brutal action.
Berserk - again mores serious series, romance develops in later half though towards the end.
Busou Renkin
Fate/Stay Night
Ga-Rei Zero, another more bloody action series but with interesting plot. Though series focus more on a friendship but main couple relationship does play a role in what is to happen.
Hakuouki - romance develops in second season or more like 3rd if you watch prequel first. I would actually start with prequel but if romance is a must then with original 1st season.
Inuyasha - longer lasting series with nice action and romance.
Katanagatari - if you don't mind lots of talking.
Mai HiME - lots of action and romance, highly recommended. Does have several fan service shots in first half but in comparison to R + V anime, it is nothing.
Otome Youkai Zakuro - something more lighthearted.
Romeo x Juliet - well that's a given.
Senjou no Valkyria: Gallian Chronicles - romance develops in later half, war orientated series.
Seirei no Moribito - these are different. They are not romance orientated though main female and male have very close relation and it isn't hard to picture them as a married couple.
The reason why I'm suggesting it is because of it's uniqueness, it isn't like most anime series out there. It has interesting plot with depth as well as nice character development for main hero.
Series are about a bodyguard Balsa who was entrusted to protect young prince who is hunted down by his own father because an evil spirit has possessed him. Series focus on their journey as well as many other things. Balsa, Tanda and Chagum start to give a massive family vibe later on so yeh do try.
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