Well, in Ouran, Haruhi was explicitly stated to be unable to sing. Hence, Sakamoto-san did not get the chance to flex her vocals. In "Maata Ashita", she only speaks (and giggles).
As for Rei, it is less of YS's art than the plotline itself. Anno-sensei, if you want us to be scared of Rei, don't make her the Woobie. Still, YS's art of her smiling in the manga is a Crowning Moment for me personally.
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