There's a lot of good VG soundtracks out there, but unanimously, I listen to Sonic the Hedgehog BGM the most frequently out of all of them.
I mostly like it for how much variety the series has and how well it can pull off each one. Such as:
and of course...
Other games with soundtracks I really like include Viewtiful Joe, Tatsunoko VS Capcom, F-Zero GX and BlazBlue.