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Infinite Stratos: Ichika x Rin
Kono kana ni hitori imouto ga iru: Shougo x Miyabi
My heart bleeds. Both twintail tsunderes lost.
OreImo: Kyousuke x Ruri
BokuTomo: Kodaka x Sena
Both in slice-of-life series involving school clubs.
Bleach: Ichigo x Rukia
Naruto: Naruto x Sakura
One Piece: Luffy x Nami
All 3 involve the lead hero and lead heroine. Though the big 3 haven't ended yet, nothing's settled in the relationships.
Yumekui Merry: Yumeji x Merry
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