I'm not sure how to find out what light novels are popular and which are not, is there a site that provides light novels' readership data >_<
Anyway, I'll mention some of what I think are popular (by looking through Japanese sites) and haven't been animated yet and haven't already been announced to get animated:
Male oriented light novels:
Bara no Maria
Ore no Imouto ga Konna ni Kawaii Wake ga Nai
Sayonara Piano Sonata
Sentou Jousai Masurawo
Tasogareiro no Uta Tsukai
Usotsuki Mii-kun to Kowareta Maa-chan
and many many more...
Female oriented light novels:
Ouran Koi Emaki
Sanzen Sekai no Karasu wo Koroshi
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