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kaze no yojimbo is the choice imo.
monster is a very good choice too but it might be a bit too long for her to stay focuse.
death note without being a bad choice requiere from the viewer to accept supernatural event in order to get into the story, so if it s the first time for your wife to watch anime it might be a bit too much, not to mention the main character even though he is charismatic is a totally despitable person.
kaze no yojimbo is a 24 episodes serie iirc so there is little chance it will start wearing on your wife's patience.
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