I think animation wise, 1999 was just better, not to mention the type of music used. Esp at the part where Killua tried to escape Phinks. In 2011, the music they used was the same one they used for Gon/Hisoka's fight, which didn't really fit the Phinks/Killua scene like it did for Gon/Hisoka. The execution of the chase was better in 1999 too, though I did like how they showed different cuts where Gon/Killua was hiding in 2011 verson.
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